Sylvia, wearing her hair in a sleek low bun, looked somewhat downcast during the conversation with her journalist husband and at times looked like she was gesturing her hand's in the air in frustration.
Outside of the cafe, Peter, 37, had his hand placed lovingly on his wife's back before she was seen talking into her phone.
Sylvia, 32, looked stylish on the streets of Double Bay wearing a rich blue midi dress with white polka dots, a maroon leather bag, and brown sandals.
Jeffreys confirmed she was leaving the Today show following Karl Stefanovics shock exit in a statement made back in December.
Jeffreys statement read: “I’ve loved and embraced every minute of my TODAY show chapter and feel humbled to have worked with so many passionate people — hosts, studio crew, cameramen and producers — who have become my great mates,
“I’m thrilled to sink my teeth into a brand new project. Opportunity often knocks when you least expect it and I’m ready to dive right in to what’s ahead of me.”