The family could be seen browsing in the aisles of the local supermarket on the island.
Pushing round a packed shopping trolley, the family picked out groceries and toys in the budget store.
While Angie wore a loose white sun dress and enormous sunglasses, the kids kept it casual in T-shirts, shorts and jeans.
The 44-year-old actress, who shares her children with ex-husband Brad Pitt, has sparked concern for her health over her gaunt appearance in the photos.
Angelina was reportedly hospitalised as a result of her anorexia as a teen, and battled with her eating disorder and self-harming in her formative years growing up in Los Angeles.
Angelina has been under stress recently, as she has combined the promotion of her movie Maleficent: Mistress of Evil along with saying goodbye to her son, Maddox, who has left for university.
Ange fought back the tears as she dropped her eldest son, Maddox Jolie-Pitt, off to college.
The 18-year-old started his first term at Yonsei University in Seoul, South Korea in August.
One lucky student managed to capture via video the moment Angelina dropped Maddox at college, where she revealed that she spent a few days in the capital Seoul, before going to the University.
In the video, taken by Jowonnn and shared via his Instagram account @xx_efu, the Oscar-winning actress looks fresh-faced and smiling while dressed in a casual black satin cami with lace detail.
In the footage, a camera-shy Maddox smiles awkwardly as he stands beside his mother.
"Nice to meet you all," Angelina says to the group of students.
An unidentified student then asks, "Miss Angelina, how long are you planning on staying in Korea this time?"
"I leave today, today's the day I drop him [Maddox] off," Angie says, before pulling a sad face.
"I'm trying not to cry."